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George Little played Haroun ed-Din in the Doctor Who television story The Crusade.
Little's first television appearance was in an episode of Maigret in 1961, after which he appeared on The Big Pull, The Avengers, The Plane Makers, The Saint, Z-Cars, Emergency – Ward 10, Softly, Softly: Taskforce, I, Claudius, When the Boat Comes In, Bergerac, Juliet Bravo, All Creatures Great and Small and The Bill. However, he is best known for playing Rev. Edward Ruskin on Emmerdale.